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Ah, that's different then - Crystic Glosscoat isn't a gelcoat, it does cure solid and epoxy can bond to it.
Breaking in moulds is definitely a thing. Though if you can get a semi-permanent tool sealer, then this will treat the chemical and physical bonding sites of a new mould in the same way that breaking them in does. So I never break in any of my new moulds, because they always get treated with a sealer first.
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