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Sort of missed this post, but it is an interesting discussion.
For me, I feel like it is sort of in the same boat as Nanotubes when it comes to how useful it is in composites. Composite structures like carbon fibre are really at their best when you minimise the influence of the resin, and maximise the influence of the fibre. Which ideally means, less resin content, higher fibre content. When you add graphene or nanotubes or any of these high performance nano materials, you are really only influencing the performance of the resin matrix and not the performance of the fibres themselves. In a high performance composite where you ideally have less than 40% resin content (and that's really on a commercial level, high end structural pre-pregs and the like are getting down below 25% resin content), say you manage to increase the strength of the resin matrix by 20%. That doesn't correspond to a 20% increase in the strength of the laminate, because the resin is less than half of the laminate. It also doesn't even necessarily correspond to a smaller fraction of the strength, depending on properties you are measuring. It is not going to heavily influence the tensile strength of the laminate for example, because tensile strength is mainly dependent on the fibre. It would have more of an influence on the compressive strength of the laminate, as the resin matrix has more influence on that property. So realistically, the actual performance increase on the laminate is quite negligible.
The argument for nanotubes has always been ''any performance increase is beneficial'', which is a fair point. And I would say if budget wasn't part of the question and you were just trying to achieve the maximum performance properties possible, then sure, probably add some nanotubes or graphene or whatever your chosen poison is and get those little gains in performance. But when you're factoring in price, the cost of the laminate vs the performance of the laminate don't really go up together in a linear fashion, so that's where the benefit of the additives becomes questionable.
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