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Cast moulds are a pretty old school, expensive way to go about it. Unimould is excellent, and is plenty rigid enough to make highly accurate moulds. Much easier to repair and restore if you ever need to as well.
You can also laminate moulds in much the same fashion as with Unimould, but using epoxy materials and woven fibreglass, for a slightly higher end mould.
For what you are doing, I would recommend Unimould everyday of the week.
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