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Have a look at a Preval sprayer system. Excellent solution for spray painting smaller objects. Even if you do decide to skip the 2k paint, you will get a much better result if you spray PVA release agent and wont have to do as much work on the mould.
There are other options that will work, like sanding the plastic smooth and spraying PVA, then refinishing the mould. Or Smooth-On 3D-XTC works ok, but isnt perfect.
Certainly if you want a professional standard part, the best way is to have a professional standard pattern - and that means painting it with 2k paints.
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