+xHave you considered infusing the molds? When I read about using jelly resin, it was unavoidable that the air pockets would ruin the mould during post cure. At least the first layer has to be absolutely perfect. And that means using a fine cloth and using thin resin. Anything much more viscous than fresh standard laminating epoxy will not wet out the cloth air free. With a fine glass cloth and black gelcoat you can see how it is getting harder to get the bubbles out as the resin starts increasing it's viscosity.
On my last try I vacuum bagged the mold after wet lay which seemed successful at removing all air, but the problem still remains that post curing off the tool (my plug was mdf and duratec) seems incredibly finicky. I didn't have positive dimples in the surface of the second mold like i did the first try, but the surface still didn't stay perfect through post cure, just kind of a wiggly surface. With another attempt of doing it on a proper tooling board plug and post cure on the plug, I could probably get the results I'm looking for, but by the time i order tooling board, more surface coat, etc., it'll cost just as much as milling these out of aluminum which is a process Im familiar with and will work perfect at making an excellent mold. Nothing can really go wrong.